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      Addressable metasurfaces for dynamic holography and optical information encryption

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          Abstract

          We present addressable plasmonic metasurfaces for optical information encryption and holography.

          Abstract

          Metasurfaces enable manipulation of light propagation at an unprecedented level, benefitting from a number of merits unavailable to conventional optical elements, such as ultracompactness, precise phase and polarization control at deep subwavelength scale, and multifunctionalities. Recent progress in this field has witnessed a plethora of functional metasurfaces, ranging from lenses and vortex beam generation to holography. However, research endeavors have been mainly devoted to static devices, exploiting only a glimpse of opportunities that metasurfaces can offer. We demonstrate a dynamic metasurface platform, which allows independent manipulation of addressable subwavelength pixels at visible frequencies through controlled chemical reactions. In particular, we create dynamic metasurface holograms for advanced optical information processing and encryption. Plasmonic nanorods tailored to exhibit hierarchical reaction kinetics upon hydrogenation/dehydrogenation constitute addressable pixels in multiplexed metasurfaces. The helicity of light, hydrogen, oxygen, and reaction duration serve as multiple keys to encrypt the metasurfaces. One single metasurface can be deciphered into manifold messages with customized keys, featuring a compact data storage scheme as well as a high level of information security. Our work suggests a novel route to protect and transmit classified data, where highly restricted access of information is imposed.

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          Most cited references27

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          From metamaterials to metadevices.

          Metamaterials, artificial electromagnetic media that are structured on the subwavelength scale, were initially suggested for the negative-index 'superlens'. Later metamaterials became a paradigm for engineering electromagnetic space and controlling propagation of waves: the field of transformation optics was born. The research agenda is now shifting towards achieving tunable, switchable, nonlinear and sensing functionalities. It is therefore timely to discuss the emerging field of metadevices where we define the devices as having unique and useful functionalities that are realized by structuring of functional matter on the subwavelength scale. In this Review we summarize research on photonic, terahertz and microwave electromagnetic metamaterials and metadevices with functionalities attained through the exploitation of phase-change media, semiconductors, graphene, carbon nanotubes and liquid crystals. The Review also encompasses microelectromechanical metadevices, metadevices engaging the nonlinear and quantum response of superconductors, electrostatic and optomechanical forces and nonlinear metadevices incorporating lumped nonlinear components.
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            Dispersionless phase discontinuities for controlling light propagation.

            Ultrathin metasurfaces consisting of a monolayer of subwavelength plasmonic resonators are capable of generating local abrupt phase changes and can be used for controlling the wavefront of electromagnetic waves. The phase change occurs for transmitted or reflected wave components whose polarization is orthogonal to that of a linearly polarized (LP) incident wave. As the phase shift relies on the resonant features of the plasmonic structures, it is in general wavelength-dependent. Here, we investigate the interaction of circularly polarized (CP) light at an interface composed of a dipole antenna array to create spatially varying abrupt phase discontinuities. The phase discontinuity is dispersionless, that is, it solely depends on the orientation of dipole antennas, but not their spectral response and the wavelength of incident light. By arranging the antennas in an array with a constant phase gradient along the interface, the phenomenon of broadband anomalous refraction is observed ranging from visible to near-infrared wavelengths. We further design and experimentally demonstrate an ultrathin phase gradient interface to generate a broadband optical vortex beam based on the above principle.
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              Electromagnetic reprogrammable coding-metasurface holograms

              Metasurfaces have enabled a plethora of emerging functions within an ultrathin dimension, paving way towards flat and highly integrated photonic devices. Despite the rapid progress in this area, simultaneous realization of reconfigurability, high efficiency, and full control over the phase and amplitude of scattered light is posing a great challenge. Here, we try to tackle this challenge by introducing the concept of a reprogrammable hologram based on 1-bit coding metasurfaces. The state of each unit cell of the coding metasurface can be switched between ‘1’ and ‘0’ by electrically controlling the loaded diodes. Our proof-of-concept experiments show that multiple desired holographic images can be realized in real time with only a single coding metasurface. The proposed reprogrammable hologram may be a key in enabling future intelligent devices with reconfigurable and programmable functionalities that may lead to advances in a variety of applications such as microscopy, display, security, data storage, and information processing.
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                Author and article information

                Journal
                Sci Adv
                Sci Adv
                SciAdv
                advances
                Science Advances
                American Association for the Advancement of Science
                2375-2548
                June 2018
                15 June 2018
                : 4
                : 6
                : eaar6768
                Affiliations
                [1 ]Max Planck Institute for Intelligent Systems, Heisenbergstrasse 3, 70569 Stuttgart, Germany.
                [2 ]School of Electronic Information, Wuhan University, Wuhan 430072, China.
                [3 ]Kirchhoff Institute for Physics, University of Heidelberg, Im Neuenheimer Feld 227, 69120 Heidelberg, Germany.
                [4 ]School of Physics and Astronomy, University of Birmingham, Birmingham B15 2TT, UK.
                Author notes
                [* ]Corresponding author. Email: laura.liu@ 123456is.mpg.de (N.L.); s.zhang@ 123456bham.ac.uk (S.Z.)
                Author information
                http://orcid.org/0000-0001-7891-3588
                http://orcid.org/0000-0002-0507-1065
                http://orcid.org/0000-0002-3226-4735
                http://orcid.org/0000-0003-4556-2333
                http://orcid.org/0000-0001-5831-3382
                Article
                aar6768
                10.1126/sciadv.aar6768
                6003725
                29922715
                46ff039c-52e2-4cb2-aced-36fc8be6f491
                Copyright © 2018 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC).

                This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license, which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited.

                History
                : 07 December 2017
                : 04 May 2018
                Funding
                Funded by: the European Research Council (ERC Dynamic Nano and ERC Topological) grants;
                Funded by: by the Sofja Kovalevskaja grant from the Alexander von Humboldt-Foundation;
                Categories
                Research Article
                Research Articles
                SciAdv r-articles
                Optics
                Physics
                Physics
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