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      Polydopamine Surface Chemistry: A Decade of Discovery

      1 , 2 , 3 , 4 , 5
      ACS Applied Materials & Interfaces
      American Chemical Society (ACS)

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          Abstract

          <p class="first" id="P1">Polydopamine is one of the simplest and most versatile approaches to functionalizing material surfaces, having been inspired by the adhesive nature of catechols and amines in mussel adhesive proteins. Since its first report in 2007, a decade of studies on polydopamine molecular structure, deposition conditions, and physicochemical properties have ensued. During this time, potential uses of polydopamine coatings have expanded in many unforeseen directions, seemingly only limited by the creativity of researchers seeking simple solutions to manipulating surface chemistry. In this review, we describe the current state of the art in polydopamine coating methods, describe efforts underway to uncover and tailor the complex structure and chemical properties of polydopamine, and identify emerging trends and needs in polydopamine research, including the use of dopamine analogs, nitrogen-free polyphenolic precursors, and improvement of coating mechanical properties. </p><p id="P2"> <div class="figure-container so-text-align-c"> <img alt="" class="figure" src="/document_file/9ecbe272-2443-4166-a8a0-c06b2932d0e9/PubMedCentral/image/nihms-997820-f0001.jpg"/> </div> </p>

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          Author and article information

          Journal
          ACS Applied Materials & Interfaces
          ACS Appl. Mater. Interfaces
          American Chemical Society (ACS)
          1944-8244
          1944-8252
          February 13 2018
          March 07 2018
          February 21 2018
          March 07 2018
          : 10
          : 9
          : 7523-7540
          Affiliations
          [1 ]Department of Carbon Fusion Engineering, Wonkwang University, Iksan, Jeonbuk 54538, South Korea
          [2 ]Departments of Bioengineering and Materials Science and Engineering, University of California, Berkeley, 210 Hearst Mining Building, Berkeley, California 94720-1760, United States
          [3 ]Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, United States
          [4 ]Department of Chemistry, Korea Advanced Institute of Science and Technology (KAIST), 291 University Road, Daejeon 34141, South Korea
          [5 ]Center for Nature-inspired Technology (CNiT), KAIST Institute of NanoCentury, 291 University Road, Daejeon 34141, South Korea
          Article
          10.1021/acsami.7b19865
          6320233
          29465221
          e9e22532-ca9f-4795-8ca1-e96e99cba445
          © 2018
          History

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