Chalcogenide Glass-Fiber-Based Mid-IR Sources and Applications

We have synthesized a series of chalcogenide glasses from the As-S-Se system that is designed to have strong nonlinearities. Measurements reveal that many of these glasses offer optical Kerr nonlinearities greater than 400 times that of fused silica at 1.25 and 1.55mum and figures of merit for all-optical switching greater than 5 at 1.55mum .

We demonstrate low-threshold supercontinuum generated in a highly nonlinear arsenic selenide chalcogenide nanowire with tailored dispersion. The tapered submicrometer chalcogenide fiber exhibits an ultrahigh nonlinearity, n(2) approximately 1.1x10(-17) m(2)/W and an effective mode area of 0.48 mum(2), yielding an effective nonlinearity of gamma approximately 93.4 W/m, which is over 80,000 times larger than standard silica single-mode fiber at a wavelength of approximately 1550 nm. This high nonlinearity, in conjunction with the engineered anomalous dispersion, enables low-threshold soliton fission leading to large spectral broadening at a dramatically reduced peak power of several watts, corresponding to picojoule energy.