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      Standard Practices of Reticular Chemistry

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          Abstract

          Reticular chemistry is a growing field of science with a multitude of practitioners with diverse frames of thinking, making the need for standard practices and quality indicators ever more compelling.

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          Most cited references82

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          Design and synthesis of an exceptionally stable and highly porous metal-organic framework

          O. Yaghi, Hailian Li, Mohamed Eddaoudi … (1999)
          Article 0 comments Cited 1039 times – based on 0 reviews     Review now
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            Flexible metal-organic frameworks.

            A Schneemann, V. Bon, I Schwedler … (2014)
            Advances in flexible and functional metal-organic frameworks (MOFs), also called soft porous crystals, are reviewed by covering the literature of the five years period 2009-2013 with reference to the early pertinent work since the late 1990s. Flexible MOFs combine the crystalline order of the underlying coordination network with cooperative structural transformability. These materials can respond to physical and chemical stimuli of various kinds in a tunable fashion by molecular design, which does not exist for other known solid-state materials. Among the fascinating properties are so-called breathing and swelling phenomena as a function of host-guest interactions. Phase transitions are triggered by guest adsorption/desorption, photochemical, thermal, and mechanical stimuli. Other important flexible properties of MOFs, such as linker rotation and sub-net sliding, which are not necessarily accompanied by crystallographic phase transitions, are briefly mentioned as well. Emphasis is given on reviewing the recent progress in application of in situ characterization techniques and the results of theoretical approaches to characterize and understand the breathing mechanisms and phase transitions. The flexible MOF systems, which are discussed, are categorized by the type of metal-nodes involved and how their coordination chemistry with the linker molecules controls the framework dynamics. Aspects of tailoring the flexible and responsive properties by the mixed component solid-solution concept are included, and as well examples of possible applications of flexible metal-organic frameworks for separation, catalysis, sensing, and biomedicine.
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              Industrial applications of metal-organic frameworks.

              Alexander U. Czaja, Natalia Trukhan, Ulrich Müller (2009)
              New materials are prerequisite for major breakthrough applications influencing our daily life, and therefore are pivotal for the chemical industry. Metal-organic frameworks (MOFs) constitute an emerging class of materials useful in gas storage, gas purification and separation applications as well as heterogeneous catalysis. They not only offer higher surface areas and the potential for enhanced activity than currently used materials like base metal oxides, but also provide shape/size selectivity which is important both for separations and catalysis. In this critical review an overview of the potential applications of MOFs in the chemical industry is presented. Furthermore, the synthesis and characterization of the materials are briefly discussed from the industrial perspective (88 references).
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                Author and article information

                Journal
                Journal ID (nlm-ta): ACS Cent Sci
                Journal ID (iso-abbrev): ACS Cent Sci
                Journal ID (publisher-id): oc
                Journal ID (coden): acscii
                Title: ACS Central Science
                Publisher: American Chemical Society
                ISSN (Print): 2374-7943
                ISSN (Electronic): 2374-7951
                Publication date (Electronic): 08 July 2020
                Publication date (Print): 26 August 2020
                Volume: 6
                Issue: 8
                Pages: 1255-1273
                Affiliations
                [† ]Department of Chemistry, University of California-Berkeley, Kavli Energy Nanoscience Institute at UC Berkeley , Berkeley, California 94720, United States
                [§ ]EMAT, University of Antwerp , Groenenborgerlaan 171, 2020 Antwerp, Belgium
                [⊥ ]BCMaterials, Basque Center for Materials, UPV/EHU Science Park , 48940 Leioa, Spain
                [4]Ikerbasque , Basque Foundation for Science, 48013, Bilbao, Spain
                [∥ ]Instituto de Ciencia de Materiales de Madrid (ICMM)—Consejo Superior de Investigaciones Científicas (CSIC) , C/Sor Juana Ineś de la Cruz, 3, Madrid 28049, Spain
                [∇ ]Department of Chemistry and Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, iChEM (Collaborative Innovation Center of Chemistry for Energy Materials), Fudan University , Shanghai 200433, China
                [° ]Department of Chemistry, Minnesota Supercomputing Institute, and Chemical Theory Center, University of Minnesota , Minneapolis, Minnesota 55455, United States
                Author notes
                [* ](C.G.) Email: cgropp@ 123456berkeley.edu .
                [* ](F.G.) Email: gandara@ 123456icmm.csic.es .
                [* ](Q.L.) Email: qwli@ 123456fudan.edu.cn .
                [* ](L.G.) Email: gagliard@ 123456umn.edu .
                [* ](O.M.Y.) Email: yaghi@ 123456berkeley.edu .
                Article
                DOI: 10.1021/acscentsci.0c00592
                PMC ID: 7453418
                PubMed ID: 32875067
                SO-VID: 375f3a3e-6e38-4329-8bea-2b78b0d5ddd4
                Copyright © Copyright © 2020 American Chemical Society
                License:

                This is an open access article published under an ACS AuthorChoice License, which permits copying and redistribution of the article or any adaptations for non-commercial purposes.

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                Subject: In Focus
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                document-id-old-9 oc0c00592
                document-id-new-14 oc0c00592
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