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      Superfluid stiffness of a KTaO 3-based two-dimensional electron gas

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          Abstract

          After almost twenty years of intense work on the celebrated LaAlO 3/SrTiO 3system, the recent discovery of a superconducting two-dimensional electron gas (2-DEG) in (111)-oriented KTaO 3-based heterostructures injects new momentum to the field of oxides interface. However, while both interfaces share common properties, experiments also suggest important differences between the two systems. Here, we report gate tunable superconductivity in 2-DEGs generated at the surface of a (111)-oriented KTaO 3 crystal by the simple sputtering of a thin Al layer. We extract the superfluid stiffness of the 2-DEGs and show that its temperature dependence is consistent with a node-less superconducting order parameter having a gap value larger than expected within a simple BCS weak-coupling limit model. The superconducting transition follows the Berezinskii-Kosterlitz-Thouless scenario, which was not reported on SrTiO 3-based interfaces. Our finding offers innovative perspectives for fundamental science but also for device applications in a variety of fields such as spin-orbitronics and topological electronics.

          Abstract

          Heterostructures based on (111)-oriented KTaO 3crystals are a new platform for studying oxide interfaces. Gate-tunable superconductivity in 2D electron gases at the surface of (111)-oriented KTaO 3is now reported, with the superconducting transition being of the Berezinskii-Kosterlitz-Thouless type.

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          Most cited references48

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          Ordering, metastability and phase transitions in two-dimensional systems

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            Electric field control of the LaAlO3/SrTiO3 interface ground state.

            Interfaces between complex oxides are emerging as one of the most interesting systems in condensed matter physics. In this special setting, in which translational symmetry is artificially broken, a variety of new and unusual electronic phases can be promoted. Theoretical studies predict complex phase diagrams and suggest the key role of the charge carrier density in determining the systems' ground states. A particularly fascinating system is the conducting interface between the band insulators LaAlO(3) and SrTiO(3) (ref. 3). Recently two possible ground states have been experimentally identified: a magnetic state and a two-dimensional superconducting condensate. Here we use the electric field effect to explore the phase diagram of the system. The electrostatic tuning of the carrier density allows an on/off switching of superconductivity and drives a quantum phase transition between a two-dimensional superconducting state and an insulating state. Analyses of the magnetotransport properties in the insulating state are consistent with weak localization and do not provide evidence for magnetism. The electric field control of superconductivity demonstrated here opens the way to the development of new mesoscopic superconducting circuits.
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              Dynamics of superfluid films

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                Author and article information

                Contributors
                nicolas.bergeal@espci.fr
                Journal
                Nat Commun
                Nat Commun
                Nature Communications
                Nature Publishing Group UK (London )
                2041-1723
                8 August 2022
                8 August 2022
                2022
                : 13
                : 4625
                Affiliations
                [1 ]GRID grid.460789.4, ISNI 0000 0004 4910 6535, Unité Mixte de Physique, CNRS, Thales, , Université Paris-Saclay, ; 1 Avenue Augustin Fresnel, 91767 Palaiseau, France
                [2 ]GRID grid.463715.2, ISNI 0000 0004 0369 2540, Laboratoire de Physique et d’Etude des Matériaux, ESPCI Paris, , PSL University, CNRS, Sorbonne Université, ; Paris, France
                [3 ]GRID grid.503243.3, Laboratoire de Physique des Solides, , Université Paris-Saclay, ; CNRS UMR 8502, 91405 Orsay, France
                [4 ]GRID grid.7841.a, Department of Physics and ISC-CNR, , Sapienza University of Rome, ; Rome, Italy
                Author information
                http://orcid.org/0000-0002-1521-8497
                http://orcid.org/0000-0002-5843-187X
                http://orcid.org/0000-0002-6091-3552
                http://orcid.org/0000-0002-6704-3422
                http://orcid.org/0000-0002-9016-5305
                Article
                32242
                10.1038/s41467-022-32242-y
                9360446
                35941153
                0fab3af7-c9ce-4e66-b1c9-70640864c25b
                © The Author(s) 2022

                Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.

                History
                : 18 February 2022
                : 21 July 2022
                Funding
                Funded by: FundRef https://doi.org/10.13039/501100001665, Agence Nationale de la Recherche (French National Research Agency);
                Award ID: ANR-19-CE47-0006
                Award Recipient :
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                © The Author(s) 2022

                Uncategorized
                superconducting properties and materials,surfaces, interfaces and thin films

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